No, I do not think that would work as a general rule of thumb. You really need to tailor this to the particular tire and your driving style. Running a very high pressure, that is near the limit for the tire, will produce a stiffening on the sidewall but at the cost of the center of the tread for higher tire wear. Over inflation produces those sample wear patterns you see in photos at the tire stores where the middle of the tire is worn out to a concave extent.
So, if the tire tends to roll under, that is the sidewall is not as stiff as you need for your driving style, you might want to run the pressure higher and try it. But if the tire is sliding out on you, you might want to try decreasing the pressure a bit to get a wider contact patch. Overdoing it in either direction will produce undesirable effects, however, sometimes directly opposite of what you are trying to produce.
Basically, you need to experiment. I tend to go up and down in 2 psi increments and then run trials on the same road at about the same speeds to see what happens. And it helps if the outdoor temp is about the same also, but if not, you want to get the tires well warmed up beforehand as they will then vary a lot less, so a good drive before starting your testing helps.
pax, smn